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68 4 Relaxation of Spin-State Equilibria of Metal Complexes in Solution . . . . . 1 Complexes of Iron(II) . . . . . . . . . . . . . . . . . . 2 Complexes of Iron(III) . . . . . . . . . . . . . . . . . 3 Complexes of Cobalt(II) . . . . . . . . . . . . . . . . . 74 74 79 82 5 Consequences with Respect to the Energetic and Molecular Properties of the Activated Complex from Absolute Reaction Rate Theory . . . . .
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4 2,6-Diacetylpyridine Bis( Thiosemicarbazones ) and Bis ( $-Alkyldithiocarbazates ) There have been no reports of cobalt(III) complexes of these potentially pentadentate ligands. 5 2-Acetylpyridine N-Oxide Thiosemicarbazones and S-Alkyldithiocarbazates Brown [Co(24-H)2]A (A = C10~, NO3) and [Co(24) (24-H)][CoA4] (A = C1, Br) have been isolated  and the cobalt(III) centers have B and Dq in the range 430-580 cm- 1 and 2070-2320 cm- 1, respectively. These complexes have greater covalency and a weaker ligand field than the analogous 2-acetylpyridine 4N-alkylthiosemicarbazone complexes.